Sujeet Kumar, Hariklia Dris Reitz, Xi-angxin Bi and Nobuyuki Kambe (together “Kumar”) appeal the decision of the Board of Patent Appeals and Interferences of the Patent and Trademark Office, rejecting claims 1-3, 5-16, and 19-22 of patent application Serial No. 09/136,483 entitled “Aluminum Oxide Particles” as obvious under 35 U.S.C. § 103. We vacate the Board’s decision and remand for further proceedings.
BACKGROUND
The claims of Kumar’s patent application are directed to aluminum oxide particles of submicron (nanometer) size, 1 having a specified size range and size distribution. The specification describes the production of the particles by laser pyrolysis, but the claims at issue are directed to the particles themselves, independent of their method of production. Due to their very small size and high degree of uniformity, the particles are described as well suited for use in polishing compositions.
The examiner had rejected all of the product claims, and on appeal the Board treated claims 1 and 19 as representative. Process claims have been allowed, and are not at issue. Kumar agrees that all of the claims on appeal rise or fall with claims 1 and 19.
1. A collection of particles comprising aluminum oxide, the collection of particles having
' an average diameter of primary particles from about 5 nm to about 500 nm and
less than about one in 106 particles have a diameter greater than about three times the average diameter of the collection of particles.
*1364 19. A collection of particles comprising aluminum oxide, the collection of particles having
an average diameter from about 5 nm to about 500 nm and
a distribution of particle sizes such that at least about 95 percent of the particles have a diameter greater than about 40 percent of the average diameter and less than about 160 percent of the average diameter.
The Board held the claims unpatentable on the ground of obviousness in view of U.S. Patent No. 5,389,194 (the Rostoker patent), which shows aluminum oxide particles of nanometer size. The Board found that the particle sizes and size distributions 2 of the Rostoker particles and of Kumar’s claimed particles are overlapping. Kumar concedes that the Rostoker particles overlap the Kumar particles in average particle size, but argues that they do not overlap in particle size distribution. The appeal relates primarily to the Board’s procedure, wherein the values deemed to overlap appear for the first time in the Board’s decision. Kumar states that he was unfairly precluded from replying to this evidence, and that the Board improperly refused to consider the responsive evidence submitted with Ku-mar’s request for reconsideration.
The Board’s calculations were derived from the Rostoker reference, which describes aluminum oxide having a particle size and size distribution as follows:
According to the invention, the alpha aluminum oxide particles used for polishing exhibit the following characteristics. Preferably, the particle size is “X” nm, and the distribution of particle sizes is controlled to within “Y” nm, and the particles used for polishing are “Z” percent (%) in the alpha phase, where:
“X” is 10-100 nm, such as 10, 20, 30, 40 or 50 nm, and is preferably no greater than 50 nm; and
“Y” is approximately “P” percent of “X”, where “P” is 10%, 20%, 30%, 40% or 50%, and is preferably no greater than 50% to ensure a narrow (Gaussian) distribution of particle sizes about “X”;
“Z” is at least 50%, including at least 60%, 70%, 80% and 90%, and as high as 100%.
A quality factor “Q” is inversely related to “Y”, and is a measure of the distribution of particle sizes. “Q” can be calculated as the concentration of particles at the desired size “X”, divided by the range of sizes of particles at 3 db (decibels) lower than “X”. Preferably, the size distribution of alpha aluminum oxide particles used for polishing exhibits a “Q” of at least 10, including 10, 50, 100, 500, 1000, 5000, or 10,000 (“Q” is dimensionless).
Rostoker patent, col. 7, lines 4-27. The Board selected “X” and “P” values in the range disclosed by Rostoker, 10 nm and 10% respectively, to calculate a “Y” value of 1 nm (10 nm times 10% equals 1 nm), within which Rostoker’s size distribution is controlled; this results in a particle size distribution range of 9-11 nm (10 nm ± 1). The Board found that this distribution range overlaps with the range in Kumar’s claim 1, which the Board calculated to be 0-30 nm based on a particle size distribution controlled to within three times the average diameter (10 nm times 3 equals 30 nm). Thus the Board found that the Ros-toker and Kumar distributions overlap.
*1365 Similarly, the Board selected “X” and “P” values in the range described by Ros-toker, to calculate a “Y” value of 5 nm (10 nm times 50% equals 5 nm); this results in a Rostoker distribution range of 5-15 nm (10 nm ± 5). The Board found that this range overlaps with the range in Kumar’s claim 19, which the Board calculated to be 4-16 nm based on the Kumar particle size distribution controlled to within 40-160% of the average diameter (10 nm times 40% and 160% equals 4 and 16 nm, respectively). The Board held that these overlapping values, and others shown by its calculations, established a prima facie case of obviousness of the Kumar particles.
These calculations had' not been made by the examiner, and according to the record were not presented during the argument of the appeal to the Board. The Board apparently made these calculations during its decision of the appeal. The Board included these calculations in an Appendix to its decision, holding that they support a
prima facie
case of obviousness and that Kumar’s evidence had not rebutted the
prima facie
case. Kumar’s evidence included a declaration by co-inventor Dr. Kambe to the effect that Rostoker does not enable one of ordinary skill in the field of the invention to produce particles having Kumar’s size range and distribution. Kumar cited
Beckman Instruments, Inc. v. LKB Produkter AB,
Kumar requested Board reconsideration, submitting the declaration of Dr. Ra-jiv Singh, Professor of Materials Science and Engineering at the University of Florida at Gainesville. Professor Singh explained that Rostoker’s “Q” value defines size distribution, and criticized Rostoker’s description of the “Q” value as internally inconsistent and not in conformity with standard representations of distribution functions. Professor Singh. pointed out that Rostoker stated that he used the manufacturing method of Siegel, U.S. Patent No. 5,128,081, and opined that Siegel does not produce submicron particles. The Board refused to consider Professor Singh’s declaration, ruling that Kumar had not shown good and sufficient reason why it was not earlier presented.
Kumar appeals, stating that a prima facie case of obviousness was not established, or if established was rebutted. Ku-mar objects to the tardy submission of the Board’s calculations and states that he was entitled to consideration of Professor Singh’s evidence. Kumar argues that the Singh evidence rebuts the prima facie case and that the Board should have either considered it or remanded to the examiner for that purpose.
DISCUSSION
Determination of obviousness under 35 U.S.C. § 103 is a legal conclusion based on underlying facts.
Graham v. John Deere Co.,
During examination, the examiner bears the initial burden of establishing a
prima facie
case of obviousness.
Oetiker,
A
A
prima facie
case of obviousness may be made when the only difference from the prior art is a difference in the range or value of a particular variable.
In re Peterson,
Kumar argues that Rostoker’s description of its particles is too indefinite to support any particular distribution of particle sizes. Kumar states that a skilled artisan would not understand Rostoker’s “Y” variable to have the values that the Board calculated because Rostoker, in addition to stating that “Y” is approximately “P” percent of “X,” requires that its particles meet a quality factor “Q” that is inversely related to “Y.” Kumar argues that this renders the calculation of “Y” more complex than the Board’s simplified calculation, and that Rostoker does not disclose the values the Board calculated and then used to conclude that Kumar’s size distribution overlaps with that of Rostoker. Kumar also states that the Board should have provided an opportunity to support this argument with evidence showing that the Rostoker teachings do not support the Board’s sua sponte calculations. Kumar states that the Singh declaration establishes the indefiniteness of the Rostoker reference, and challenges the assumptions underlying the Board’s calculations.
The PTO responds that Rostoker’s quality factor “Q” describes the extent to which his particle size distribution is controlled to within certain limits of the target particle size. The PTO suggests that Q is calculated as follows: Rostoker calls for the division of the amount of particles at the desired size X, by the amount of particles at a size 3 decibels (“db”) from X. To find a value 3 db from X, which the Board labels “A,” one must solve the logarithmic function, 10 log (X/A) = 3 db. The PTO solves this function and finds that if log (X/A) = 3/10, then X/A = 103/1°, and thus X/A = 2, and A = X/2. This means that a value that is 3 db lower than X is X/2 or 50% of X. Thus the PTO states that the quality factor Q merely describes the extent to which the particles are within 50% and 150% of the target particle size. For example, the “Q” value of 10,000 in the Rostoker reference indicates a high quality *1367 product in which 10,000 particles are of the target size for every particle at 50% or 150% of the target size. According to the PTO, rather than making indefinite the values for “X” and “Y” as shown by Ros-toker and the ranges of those values, the “Q” factor provides an independent description of Rostoker’s particle size distribution.
The PTO also responds that the Board was correct in refusing to consider the Singh declaration because its execution date shows that it was prepared before the Board issued its initial decision, and thus could have been earlier presented. Kumar states that the Singh declaration was prepared for use in a different patent application, and that its relevance to this application became manifest only after the Board’s decision.
The values identified by the Board’s calculations were not contained in the prior art or any examination record, but appeared for the first time in the Board’s opinion. Although the PTO argues that the calculations the Board included in its decision were not new evidence, but simply an additional explanation of the Board’s decision, these values produced and relied on by the Board had not previously been identified by the examiner or the Board. Kumar was entitled to respond to these calculations, and the Board committed procedural error in refusing to consider the evidence proffered in response.
See In re DeBlauwe,
Instead of basing its decision on the values directly disclosed by Rostoker, the Board “went off on its own in considering the differences” between Rostoker and the Kumar invention,
see In re Eynde,
In accordance with the Administrative Procedure Act, the agency must assure that an applicant’s petition is fully and fairly treated at the administrative level, without interim need for judicial intervention.
See Dickinson v. Zurko,
When a rejection for obviousness is based on overlapping values in the prior art, identification of the values deemed to overlap is material to the rejection. In this case the overlapping values were identified for the first time in the decision of the Board, and are not themselves set forth in Rostoker or any other reference.
*1368
In calculating the overlapping values, the Board found facts not found by the examiner regarding the differences between the prior art and the claimed invention, which in fairness required an opportunity for response.
See In re Kronig,
We conclude that the Board’s calculations and its decision based thereon constituted a new ground of rejection, and should have been so treated.
See In re Waymouth,
B
Kumar also argues that even if a prim a facie case of obviousness were established, Kumar rebutted that case with evidence and argument that Rostoker did not enable the Kumar product, and that the Board erred in refusing to consider the rebuttal evidence.
An applicant may rebut a
prima facie
case of obviousness by providing a “showing of facts supporting the opposite conclusion.” Such a showing dissipates the
prima facie
holding and requires the examiner to “consider all of the evidence anew.”
Piasecki,
Although published subject matter is “prior art” for all that it discloses, in order to render an invention unpatentable for obviousness, the prior art must enable a person of ordinary skill to make and use the invention.
Beckman Instruments,
The applicant has the burden of coming forward with evidence in rebuttal, when the prior art includes a method that appears, on its face, to be capable of producing the claimed composition. This burden may be met by presenting sufficient reason or authority or evidence, on the facts of the case, to show that the prior art method would not produce or would not be expected to produce the claimed subject matter. Since Rostoker states that its particles were made by the method shown in the Siegel patent, it was reasonable for Kumar to argue that the Siegel process would not produce Kumar’s particles. Ku-
*1369
mar’s argument was supported by the declarations of Drs. Kambe and Singh. Whether these expert declarations are sufficient, without experimental data or other evidence, is a question of fact to be determined on the record. Although the PTO now argues that the Singh declaration is insufficient, the Board erred in refusing to consider the Singh declaration, for Kumar correctly observed that the issue was not presented until the Board made its
sua sponte
calculations of particle size distribution. The Board’s calculations raised new issues regarding enablement because they suggest particle size distributions Rostoker should be enabled to attain. In addition, although the Board found the Kambe declaration conclusory and insufficient to rebut the
prima facie
case of obviousness, this declaration must be reevaluated in light of the Singh declaration.
See Rinehart,
The PTO argues that as long as Rostoker enables the Rostoker invention, Rostoker renders the Kumar invention obvious, even if Kumar shows that Rostoker does not enable the Kumar invention. That is incorrect. To render a later invention un-patentable for obviousness, the prior art must enable a person of ordinary skill in the field to make and use the later invention.
Beckman Instruments, Inc.,
After the Board adduced its calculations of particle size and distribution, Kumar was entitled to offer evidence in rebuttal, for consideration by the Board or on return to an examiner. The entirety of the evidence must be reviewed in order to determine whether the claimed invention as a whole would have been obvious to a person of ordinary skill in the field.
See Rinehart,
CONCLUSION
In view of our holding that Kumar was entitled to respond to the evidence adduced sua sponte by the Board, we vacate the Board’s decision and remand for appropriate further proceedings.
VACATED AND REMANDED
Notes
. One micron equals 1,000 nanometers (nm).
. The parties explain the difference between average particle size and particle size distribution with an analogy using balls: a collection of (1) softballs, baseballs and tennis balls may have the same average size as a collection of (2) basketballs, baseballs and golf balls, but group (2) has a larger size distribution.
